Rolf A T M van Benthem
Overview
Explore the profile of Rolf A T M van Benthem including associated specialties, affiliations and a list of published articles.
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25
Citations
141
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Recent Articles
1.
van Leuken S, van Gorp J, van Benthem R, Vis M, Tuinier R
Chemphyschem
. 2024 Oct;
25(22):e202400206.
PMID: 39447082
Mixing different aliphatic polyamides provides opportunities to tune and optimize the properties of these semicrystalline polycondensates. Combining experiment and theory, we predict and explain the miscibility of aliphatic polyamide mixtures....
2.
van den Akker W, van Benthem R, Voets I, van Hest J
ACS Appl Mater Interfaces
. 2024 Apr;
16(15):19642-19650.
PMID: 38569110
The fabrication of a soft actuator with a dampened actuation response is presented. This was achieved via the incorporation into an actuating hydrogel of urease-loaded pH-responsive bicontinuous nanospheres (BCNs), whose...
3.
Wink R, Majumdar S, van Benthem R, Heuts J, Sijbesma R
Polym Chem
. 2023 Nov;
14(37):4294-4302.
PMID: 38013800
Neighboring group assisted rearrangement substantially increases relaxation rates in dynamic covalent networks, allowing easier (re)processing of these materials. In this work, we introduce a dynamic covalent network with anionic phosphate...
4.
Zhang H, van Hertrooij A, Schnitzer T, Chen Y, Majumdar S, van Benthem R, et al.
Macromolecules
. 2023 Aug;
56(16):6452-6460.
PMID: 37637305
In dynamic polyamide networks, 1,2,4,5-benzene tetraamide (B4A) units act simultaneously as a dynamic covalent cross-linker and as supramolecular stacking motif. This results in materials with a rubbery plateau modulus that...
5.
van den Akker W, Wu H, Welzen P, Friedrich H, Abdelmohsen L, van Benthem R, et al.
J Am Chem Soc
. 2023 Mar;
PMID: 36995949
We demonstrate the construction of pH-responsive bicontinuous nanospheres (BCNs) with nonlinear transient permeability and catalytic activity. The BCNs were assembled from amphiphilic block copolymers comprising pH-responsive groups and were loaded...
6.
Maddala S, Liao W, Joosten R, Soleimani M, Tuinier R, Friedrich H, et al.
Commun Chem
. 2023 Jan;
4(1):160.
PMID: 36697574
Polyamines play a major role in biosilicification reactions in diatoms and sponges. While the effects of polyamines on silicic acid oligomerization and precipitation are well known, the impact of polyamines...
7.
Majumdar S, Zhang H, Soleimani M, van Benthem R, Heuts J, Sijbesma R
ACS Macro Lett
. 2022 Jun;
9(12):1753-1758.
PMID: 35653678
Dynamic covalent networks are a class of polymeric materials that combine the merits of classical thermosets and thermoplastics, in terms of mechanical properties and reprocessability, in one material. Various dynamic...
8.
Li C, Sablong R, van Benthem R, Koning C
ACS Macro Lett
. 2022 Jun;
6(7):684-688.
PMID: 35650870
The depolymerization of poly(limonene carbonate) (PLC) initiated by 1,5,7-triazabicyclo[4.4.0]dec-5-ene (TBD) was investigated. The strong organic base TBD was capable of deprotonating the OH-terminated PLC, leading to fast degradation via backbiting...
9.
Zhang H, Majumdar S, van Benthem R, Sijbesma R, Heuts J
ACS Macro Lett
. 2022 May;
9(2):272-277.
PMID: 35638690
Dynamic covalent bonds in a polymer network lead to plasticity, reshapability, and potential recyclability at elevated temperatures in combination with solvent-resistance and better dimensional stability at lower temperatures. Here we...
10.
Soleimani M, van den Broek S, Joosten R, van Hazendonk L, Maddala S, van Breemen L, et al.
Nanomaterials (Basel)
. 2022 May;
12(9).
PMID: 35564259
Investigating and understanding the intrinsic material properties of biogenic materials, which have evolved over millions of years into admirable structures with difficult to mimic hierarchical levels, holds the potential of...