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Lee Belding

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Articles 25
Citations 242
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Recent Articles
1.
Jiang H, Underwood T, Bell J, Lei J, Gonzales J, Emge L, et al.
Proc Natl Acad Sci U S A . 2024 Jul; 121(32):e2400819121. PMID: 39074283
To test the hypothesis that an abiotic Earth and its inert atmosphere could form chemically reactive carbon- and nitrogen-containing compounds, we designed a plasma electrochemical setup to mimic lightning-induced electrochemistry...
2.
Li Y, Root S, Belding L, Park J, Yoon H, Huang C, et al.
J Phys Chem B . 2022 Dec; 127(1):407-424. PMID: 36580625
This paper describes measurements of charge transport by tunneling through molecular junctions comprising a self-assembled monolayer (SAM) supported by a template-stripped metal bottom electrode (M), which has been immersed in...
3.
Park J, Kodaimati M, Belding L, Root S, Schatz G, Whitesides G
ACS Nano . 2022 Mar; 16(3):4206-4216. PMID: 35230085
The problem this paper addresses is the origin of the hysteretic behavior in two-terminal molecular junctions made from an EGaIn electrode and self-assembled monolayers of alkanethiolates terminated in chelates (transition...
4.
Li Y, Root S, Belding L, Park J, Rawson J, Yoon H, et al.
J Am Chem Soc . 2021 Apr; 143(15):5967-5977. PMID: 33834784
This paper describes a surface analysis technique that uses the "EGaIn junction" to measure tunneling current densities ((V), amps/cm) through self-assembled monolayers (SAMs) terminated in a chelating group and incorporating...
5.
Belding L, Root S, Li Y, Park J, Baghbanzadeh M, Rojas E, et al.
J Am Chem Soc . 2021 Feb; 143(9):3481-3493. PMID: 33621090
This paper demonstrates that the molecular conformation (in addition to the composition and structure) of molecules making up self-assembled monolayers (SAMs) influences the rates of charge tunneling (CT) through them,...
6.
Park J, Belding L, Yuan L, Mousavi M, Root S, Yoon H, et al.
J Am Chem Soc . 2021 Jan; 143(4):2156-2163. PMID: 33480255
This paper addresses the mechanism for rectification in molecular tunneling junctions based on alkanethiolates terminated by a bipyridine group complexed with a metal ion, that is, having the structure Au-S(CH)BIPY-MCl...
7.
Rothemund P, Ainla A, Belding L, Preston D, Kurihara S, Suo Z, et al.
Sci Robot . 2020 Nov; 3(16). PMID: 33141749
Almost all pneumatic and hydraulic actuators useful for mesoscale functions rely on hard valves for control. This article describes a soft, elastomeric valve that contains a bistable membrane, which acts...
8.
Baghbanzadeh M, Belding L, Yuan L, Park J, Al-Sayah M, Bowers C, et al.
J Am Chem Soc . 2019 May; 141(22):8969-8980. PMID: 31072101
This Article describes the relationship between molecular structure, and the rectification of tunneling current, in tunneling junctions based on self-assembled monolayers (SAMs). Molecular dipoles from simple organic functional groups (amide,...
9.
Cafferty B, Wong A, Semenov S, Belding L, Gmur S, Huck W, et al.
J Am Chem Soc . 2019 May; 141(20):8289-8295. PMID: 31035761
How simple chemical reactions self-assembled into complex, robust networks at the origin of life is unknown. This general problem-self-assembly of dissipative molecular networks-is also important in understanding the growth of...
10.
Semenov S, Belding L, Cafferty B, Mousavi M, Finogenova A, Cruz R, et al.
J Am Chem Soc . 2018 Jul; 140(32):10221-10232. PMID: 30035540
This work describes the autocatalytic copper-catalyzed azide-alkyne cycloaddition (CuAAC) reaction between tripropargylamine and 2-azidoethanol in the presence of Cu(II) salts. The product of this reaction, tris-(hydroxyethyltriazolylmethyl)amine (N(CN)), accelerates the cycloaddition...