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Stephen M Holmes

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Articles 22
Citations 76
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Recent Articles
1.
Yang J, You M, Liu S, Deng Y, Chang X, Holmes S, et al.
Inorg Chem . 2023 Oct; 62(42):17530-17536. PMID: 37801447
Extending a selected cyanometalate block into a higher dimensional framework continues to present intriguing challenges in the fields of chemistry and material science. Here, we prepared two rope-like chain compounds...
2.
Meng L, Deng Y, Holmes S, Zhang Y
Dalton Trans . 2023 Jan; 52(6):1616-1622. PMID: 36648100
Recently, a family of [FeCo] molecular capsules that display tunable electron transfer-coupled spin transition (ETCST) behavior were reported a smart approach through Schiff-base condensation of aldehyde-functionalized 2,2-bipyridines (bpy) and 1,7-heptanediamine...
3.
Zhang Y, Ferko P, Siretanu D, Ababei R, Rath N, Shaw M, et al.
J Am Chem Soc . 2014 Oct; 136(48):16854-64. PMID: 25340715
Two structurally related and photoresponsive cyanide-bridged Fe/Co square complexes, {Fe2Co2}, are reported: {[(Tp(Me))Fe(CN)3]2[Co(bpy)2]2[(Tp(Me))Fe(CN)3]2}·12H2O (2) and {[(Tp(Me))Fe(CN)3]2[Co(bpy)2]2[BPh4]2}·6MeCN (3), where Tp(Me) and bpy are hydridotris(3-methylpyrazol-1-yl)borate and 2,2'-bipyridine, respectively. Through electrochemical and spectroscopic...
4.
Panja A, Guionneau P, Jeon I, Holmes S, Clerac R, Mathoniere C
Inorg Chem . 2012 Nov; 51(22):12350-9. PMID: 23134343
A new symmetrical tricyanide building block mer-[Fe(bbp)(CN)3](2-) [1; bbp = bis(2-benzimidazolyl)pyridine dianion] has been prepared and structurally and magnetically characterized. It forms a new low-spin meridionally capped {Fe(III)L(CN)3} fragment with...
5.
Zhang Y, Mallik U, Rath N, Clerac R, Holmes S
Inorg Chem . 2011 Sep; 50(21):10537-9. PMID: 21950315
A new tricyanoferrate(III) building block and a trinuclear single-molecule magnet derivative are described. The treatment of a 2:1 ratio of [NEt(4)][(Tp*(Bn))Fe(III)(CN)(3)]·H(2)O·MeOH [1; Tp*(Bn) = tris(3,5-dimethyl-4-benzyl)pyrazolylborate] with nickel(II) trifluoromethanesulfonate gives {[(Tp*(Bn))Fe(III)(CN)(3)](2)[Ni(II)(DMF)(4)]}·2DMF...
6.
Siretanu D, Li D, Buisson L, Bassani D, Holmes S, Mathoniere C, et al.
Chemistry . 2011 Sep; 17(42):11704-8. PMID: 21905143
No abstract available.
7.
Zhang Y, Mallik U, Clerac R, Rath N, Holmes S
Chem Commun (Camb) . 2011 Jun; 47(25):7194-6. PMID: 21625681
Two cyano-bridged single-molecule magnets of {Fe(III)(4)Ni(II)(2)} and {Fe(III)(6)Ni(II)(3)} stoichiometry are described via their magnetic properties described in the frame of geometrical core distortions and orientations of their local anisotropy axes.
8.
Tang M, Li D, Mallik U, Zhang Y, Clerac R, Yee G, et al.
Inorg Chem . 2011 Apr; 50(11):5153-64. PMID: 21520919
The syntheses, structures, and magnetic properties of a series of di- and trivalent hydridotris(3,5-dimethylpyrazol-1-yl)borate (Tp*) cyanomanganates are described. Treatment of tris(acetylacetonate)manganese(III) [Mn(acac)(3)] with KTp* and tetra(ethyl)ammonium cyanide affords [NEt(4)][(Tp*)Mn(II)(κ(2)-acac)(CN)] (1),...
9.
Zhang Y, Mallik U, Rath N, Yee G, Clerac R, Holmes S
Chem Commun (Camb) . 2010 Jun; 46(27):4953-5. PMID: 20526498
A new low symmetry octanuclear cyano-based {Fe(III)(4)Ni(II)(4)} single-molecule magnet (SMM) is described. This SMM exhibits the highest energy barrier (Delta/k(B) approximately 33 K) for magnetization reversal seen for any first-row...
10.
Tang M, Li D, Mallik U, Withers J, Brauer S, Rhodes M, et al.
Inorg Chem . 2010 May; 49(11):4753-5. PMID: 20438094
Treatment of tris(3-cyano-2,4-pentanedionato)manganese(III) with KTp*, followed by [NEt(4)]CN affords [NEt(4)][(Tp*)Mn(III)(CN)(3)] (1); subsequent treatment of 1 with divalent triflates (OTf) and 2,2'-bipyridine (bpy) affords {Mn(III)(2)M(II)(2)} complexes (M(II) = Mn, 2; Ni,...