Pieter J Smeets
Overview
Explore the profile of Pieter J Smeets including associated specialties, affiliations and a list of published articles.
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6
Citations
238
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Recent Articles
1.
Vanelderen P, Hadt R, Smeets P, Solomon E, Schoonheydt R, Sels B
J Catal
. 2013 Mar;
284(2):157-164.
PMID: 23487537
The present work highlights recent advances in elucidating the methane oxidation mechanism of inorganic Cu-ZSM-5 biomimic and in identifying the reactive intermediates that are involved. Such molecular understanding is important...
2.
Solomon E, Ginsbach J, Heppner D, Kieber-Emmons M, Kjaergaard C, Smeets P, et al.
Faraday Discuss
. 2011 Feb;
148:11-39.
PMID: 21322475
Cu/O2 intermediates in biological, homogeneous, and heterogeneous catalysts exhibit unique spectral features that reflect novel geometric and electronic structures that make significant contributions to reactivity. This review considers how the...
3.
Smeets P, Hadt R, Woertink J, Vanelderen P, Schoonheydt R, Sels B, et al.
J Am Chem Soc
. 2010 Oct;
132(42):14736-8.
PMID: 20923156
The reactive oxidizing species in the selective oxidation of methane to methanol in oxygen activated Cu-ZSM-5 was recently defined to be a bent mono(μ-oxo)dicopper(II) species, [Cu(2)O](2+). In this communication we...
4.
Smeets P, Woertink J, Sels B, Solomon E, Schoonheydt R
Inorg Chem
. 2010 Apr;
49(8):3573-83.
PMID: 20380459
Zeolites containing transition-metal ions (TMIs) often show promising activity as heterogeneous catalysts in pollution abatement and selective oxidation reactions. In this paper, two aspects of research on the TMIs Cu,...
5.
Woertink J, Smeets P, Groothaert M, Vance M, Sels B, Schoonheydt R, et al.
Proc Natl Acad Sci U S A
. 2009 Oct;
106(45):18908-13.
PMID: 19864626
Driven by the depletion of crude oil, the direct oxidation of methane to methanol has been of considerable interest. Promising low-temperature activity of an oxygen-activated zeolite, Cu-ZSM-5, has recently been...
6.
Groothaert M, Smeets P, Sels B, Jacobs P, Schoonheydt R
J Am Chem Soc
. 2005 Feb;
127(5):1394-5.
PMID: 15686370
This work reports on the capability of the O2-activated Cu-ZSM-5 and Cu-MOR zeolites to selectively convert methane into methanol at a temperature of 398 K. A strong correlation between (i)...