Jochen Autschbach
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Explore the profile of Jochen Autschbach including associated specialties, affiliations and a list of published articles.
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329
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2054
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Recent Articles
1.
Russo D, Gaiser A, Price A, Sergentu D, Wacker J, Katzer N, et al.
Science
. 2025 Feb;
387(6737):974-978.
PMID: 40014698
Interest in actinide-carbon bonds has persisted since actinide organometallics were first investigated for applications in isotope separation during the Manhattan Project. Transplutonium organometallics are rarely isolated and structurally characterized, likely...
2.
Pandey P, Zaichenko A, Smith P, Russo D, Gau M, Carroll P, et al.
Inorg Chem
. 2025 Feb;
64(7):3346-3359.
PMID: 39937136
A series of solvated complexes: [(CH)Ln(CMeR)(DME)] Ln = La, R = -Me; () Ln = Ce, R = -Me, -SiMe, -H; (, , ), [(dbCOT)Ln(CMe)(DME)] (), (dbCOT = dibenzocyclooctadienide; Ln...
3.
Hayton T, Autschbach J
Acc Chem Res
. 2025 Jan;
58(3):488-498.
PMID: 39838941
ConspectusUnderstanding f element-ligand covalency is at the center of efforts to design new separations schemes for spent nuclear fuel, and is therefore of signficant fundamental and practical importance. Considerable effort...
4.
Russo D, Branson J, Kelly S, Sen A, Gunther S, Peterson A, et al.
Chem Commun (Camb)
. 2025 Jan;
61(12):2504-2507.
PMID: 39820218
An isostructural series of four annulated actinocene complexes, M(hdcCOT) (M = Th, U, Np, Pu), is reported. The syntheses proceed through a trivalent starting material when M = U, Np,...
5.
Cao Z, Yu X, Yao Y, Autschbach J, Chen N
J Am Chem Soc
. 2025 Jan;
147(4):3584-3592.
PMID: 39813405
A thorium-carbon double bond that corresponds to the sum of theoretical covalent double bond radii has long been sought after in the study of actinide-ligand multiple bonding as a synthetic...
6.
Shakiba M, Philips A, Autschbach J, Akimov A
J Phys Chem Lett
. 2024 Dec;
16(1):153-162.
PMID: 39707977
In this work, a machine learning mapping approach for predicting the properties of atomistic systems is reported. Within this approach, the atomic orbital overlap, density, or Kohn-Sham (KS) Fock matrix...
7.
Autschbach J, Bart S, Brutchey R, Chen B, Cossairt B, Cummins C, et al.
Inorg Chem
. 2024 Dec;
63(48):22629-22638.
PMID: 39618240
No abstract available.
8.
Aguirre Quintana L, Lussier D, Wacker J, Bajaj A, Russo D, Cosby A, et al.
J Am Chem Soc
. 2024 Nov;
146(46):31671-31680.
PMID: 39500515
We report the synthesis and characterization of the macrocyclic californium derivative Na[Cf(HO)(DOTA)] (DOTA = 1,4,7,10-tetraazacyclododecane-1,4,7,10-tetraacetate), , which was studied in comparison to its dysprosium counterpart, Na[Dy(HO)(DOTA)], . Divergent spectroscopic and...
9.
Ordonez O, Yu X, Schuerlein M, Wu G, Autschbach J, Hayton T
J Am Chem Soc
. 2024 Oct;
PMID: 39371031
The reaction of [CpTh(3,3-diphenylcyclopropenyl)] (Cp = η-CH) with 1 equiv of lithium diisopropylamide (LDA) results in cyclopropenyl ring opening and formation of the thorium allenylidene complex, [Li(EtO)][CpTh(CCCPh)] ([Li(EtO)][]), in good...
10.
Branson J, Smith P, Sergentu D, Russo D, Gupta H, Booth C, et al.
J Am Chem Soc
. 2024 Sep;
146(37):25640-25655.
PMID: 39241121
The 4f orbitals of Ce(IV) have shown appreciably enhanced covalent mixing with ligand orbitals relative to those of Ce(III). Here, X-ray spectroscopy, magnetic susceptibility measurements, and theoretical methods are used...