Brian L Wadsworth
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Explore the profile of Brian L Wadsworth including associated specialties, affiliations and a list of published articles.
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11
Citations
97
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Recent Articles
1.
Reyes Cruz E, Nishiori D, Wadsworth B, Nguyen N, Hensleigh L, Khusnutdinova D, et al.
Chem Rev
. 2022 Sep;
122(21):16051-16109.
PMID: 36173689
Nature offers inspiration for developing technologies that integrate the capture, conversion, and storage of solar energy. In this review article, we highlight principles of natural photosynthesis and artificial photosynthesis, drawing...
2.
Arsenault E, Guerra W, Shee J, Reyes Cruz E, Yoneda Y, Wadsworth B, et al.
J Phys Chem Lett
. 2022 May;
13(20):4479-4485.
PMID: 35575065
Photoinduced proton-coupled electron transfer and long-range two-proton transport via a Grotthuss-type mechanism are investigated in a biomimetic construct. The ultrafast, nonequilibrium dynamics are assessed via two-dimensional electronic vibrational spectroscopy, in...
3.
Odella E, Mora S, Wadsworth B, Goings J, Gervaldo M, Sereno L, et al.
Chem Sci
. 2021 Jun;
11(15):3820-3828.
PMID: 34122850
Designing molecular platforms for controlling proton and electron movement in artificial photosynthetic systems is crucial to efficient catalysis and solar energy conversion. The transfer of both protons and electrons during...
4.
Nishiori D, Wadsworth B, Reyes Cruz E, Nguyen N, Hensleigh L, Karcher T, et al.
Photosynth Res
. 2021 May;
151(2):1-10.
PMID: 34021849
Photoelectrosynthetic materials provide a bioinspired approach for using the power of the sun to produce fuels and other value-added chemical products. However, there remains an incomplete understanding of the operating...
5.
Yoneda Y, Mora S, Shee J, Wadsworth B, Arsenault E, Hait D, et al.
J Am Chem Soc
. 2021 Feb;
143(8):3104-3112.
PMID: 33601880
Although photoinduced proton-coupled electron transfer (PCET) plays an essential role in photosynthesis, a full understanding of the mechanism is still lacking due to the complex nonequilibrium dynamics arising from the...
6.
Guerra W, Odella E, Secor M, Goings J, Urrutia M, Wadsworth B, et al.
J Am Chem Soc
. 2020 Dec;
142(52):21842-21851.
PMID: 33337139
The essential role of a well-defined hydrogen-bond network in achieving chemically reversible multiproton translocations triggered by one-electron electrochemical oxidation/reduction is investigated by using pyridylbenzimidazole-phenol models. The two molecular architectures designed...
7.
Nguyen N, Wadsworth B, Nishiori D, Reyes Cruz E, Moore G
J Phys Chem Lett
. 2020 Dec;
12(1):199-203.
PMID: 33325709
Understanding and controlling factors that restrict the rates of fuel-forming reactions are essential to designing effective catalyst-modified semiconductors for applications in solar-to-fuel technologies. Herein, we describe GaAs semiconductors featuring a...
8.
Wadsworth B, Khusnutdinova D, Urbine J, Reyes A, Moore G
ACS Appl Mater Interfaces
. 2019 Nov;
12(3):3903-3911.
PMID: 31679340
Rationally designed material interfaces offer opportunities to control matter and energy across multiple length scales, yet remain challenging to synthetically prepare. Inspired by nature, where amino acid residues and soft-material...
9.
Wadsworth B, Beiler A, Khusnutdinova D, Reyes Cruz E, Moore G
J Am Chem Soc
. 2019 Aug;
141(40):15932-15941.
PMID: 31461276
We report on the interplay between light absorption, charge transfer, and catalytic activity at molecular-catalyst-modified semiconductor liquid junctions. Factors limiting the overall photoelectrosynthetic transformations are presented in terms of distinct...
10.
Odella E, Wadsworth B, Mora S, Goings J, Huynh M, Gust D, et al.
J Am Chem Soc
. 2019 Aug;
141(36):14057-14061.
PMID: 31390197
Proton-coupled electron transfer (PCET) combines the movement of fundamental charged species to form an essential link between electron- and proton-transport reactions in bioenergetics and catalysis in general. The length scale...