Andrew M Rappe
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Explore the profile of Andrew M Rappe including associated specialties, affiliations and a list of published articles.
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148
Citations
1426
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Recent Articles
1.
Kim J, Qi Y, Kumar A, Tang Y, Xu M, Takenaka H, et al.
Nat Nanotechnol
. 2025 Feb;
PMID: 39934648
Relaxor ferroelectrics (relaxors) are a special class of ferroelectrics with polar nanodomains (PNDs), which present characteristics such as slim hysteresis loops and strong dielectric relaxation. Applications such as nanoelectromechanical systems,...
2.
Skidmore C, Spurling R, Hayden J, Baksa S, Behrendt D, Goodling D, et al.
Nature
. 2025 Jan;
637(8046):574-579.
PMID: 39779861
Proximity ferroelectricity is an interface-associated phenomenon in electric-field-driven polarization reversal in a non-ferroelectric polar material induced by one or more adjacent ferroelectric materials. Here we report proximity ferroelectricity in wurtzite...
3.
Zhou S, Rappe A
Proc Natl Acad Sci U S A
. 2024 Dec;
122(1):e2406316122.
PMID: 39739792
Ferroelectric hafnia exhibits promising robust polarization and silicon compatibility for ferroelectric devices. Unfortunately, it suffers from difficult polarization switching. Methods to enable easier polarization switching are needed, and the underlying...
4.
Hawthorne N, Broker Jr E, Bao Y, Banerjee S, Moore Q, Cardinal C, et al.
Mater Horiz
. 2024 Nov;
12(4):1179-1188.
PMID: 39588715
Using mechanical force to induce chemical reactions with two-dimensional (2D) materials provides an approach for both understanding mechanochemical processes on the molecular level, and a potential method for using mechanical...
5.
Roller D, Rappe A, Kronik L, Hellman O
J Chem Phys
. 2024 Aug;
161(7).
PMID: 39162196
The high-order finite difference real-space pseudopotential density functional theory (DFT) approach is a valuable method for large-scale, massively parallel DFT calculations. A significant challenge in the approach is the oscillating...
6.
Kim D, Woo S, Huelmo C, Park M, Schankler A, Dai Z, et al.
Nat Commun
. 2024 Jul;
15(1):6245.
PMID: 39048540
Reducing the size of perovskite crystals to confine excitons and passivating surface defects has fueled a significant advance in the luminescence efficiency of perovskite light-emitting diodes (LEDs). However, the persistent...
7.
Gallagher S, Kline J, Jahanbakhshi F, Sadighian J, Lyons I, Shen G, et al.
ACS Nano
. 2024 Jul;
18(29):19208-19219.
PMID: 38982590
Photoluminescence intermittency remains one of the biggest challenges in realizing perovskite quantum dots (QDs) as scalable single photon emitters. We compare CsPbBr QDs capped with different ligands, lecithin, and a...
8.
Fang H, Thakur A, Zahmatkeshsaredorahi A, Fang Z, Rad V, Shamsabadi A, et al.
Proc Natl Acad Sci U S A
. 2024 Jul;
121(28):e2400084121.
PMID: 38968114
MXenes have demonstrated potential for various applications owing to their tunable surface chemistry and metallic conductivity. However, high temperatures can accelerate MXene film oxidation in air. Understanding the mechanisms of...
9.
Castro-Mendez A, Jahanbakhshi F, LaFollette D, Lawrie B, Li R, Perini C, et al.
J Am Chem Soc
. 2024 Jun;
146(27):18459-18469.
PMID: 38934577
Coevaporation of formamidinium lead iodide (FAPbI) is a promising route for the fabrication of highly efficient and scalable optoelectronic devices, such as perovskite solar cells. However, it poses experimental challenges...
10.
Zhang T, Jiang Z, Rappe A
J Am Chem Soc
. 2024 May;
146(22):15488-15495.
PMID: 38776284
Recently, many topological materials have been discovered as promising electrocatalysts in chemical conversion processes and energy storage. However, it remains unclear how the topological electronic states specifically modulate the catalytic...