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Structurally-colored Adhesives for Sensitive, High-resolution, and Non-invasive Adhesion Self-monitoring

Overview
Journal Nat Commun
Specialty Biology
Date 2024 Sep 28
PMID 39341839
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Abstract

Polymeric adhesives are critical in many applications, from daily life to implantable devices and soft robotics. Monitoring adhesion in a real-time and convenient manner before premature failure is essential yet challenging. Herein, we present structurally-colored adhesives for sensitive, high-resolution, and non-invasive adhesion self-monitoring via distinct color change for detecting subtle deformation and debonding. The structurally-colored adhesives are designed by integrating one-dimensional photonic nanochains into exemplified acrylate-copolymer-based adhesives and demonstrate distinct color-changing capability through a unique tilting mechanism of nanochains under shear. Our structurally-colored adhesives can be customized as pressure-sensitive and structural adhesives, exhibiting ultrafast response (<60 ms), high sensitivity, and high resolution (~120 μm). Moreover, predicting adhesion states and premature failure can be achieved assisted by imaging systems and machine learning algorithms with an average accuracy of up to 97.2%. Our structurally-colored adhesives are expected to offer a practical paradigm for structural health monitoring in the Internet of Things era.

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