A Graph-based Modeling Framework for Tracing Hydrological Pollutant Transport in Surface Waters

Overview

Journal Comput Chem Eng

Date 2024 Jan 24

PMID 38264312

Authors

David L Cole

Gerardo J Ruiz-Mercado

Victor M Zavala

Affiliations

Soon will be listed here.

Abstract

Anthropogenic pollution of hydrological systems affects diverse communities and ecosystems around the world. Data analytics and modeling tools play a key role in fighting this challenge, as they can help identify key sources as well as trace transport and quantify impact within complex hydrological systems. Several tools exist for simulating and tracing pollutant transport throughout surface waters using detailed physical models; these tools are powerful, but can be computationally intensive, require significant amounts of data to be developed, and require expert knowledge for their use (ultimately limiting application scope). In this work, we present a graph modeling framework - which we call HydroGraphs - for understanding pollutant transport and fate across waterbodies, rivers, and watersheds. This framework uses a simplified representation of hydrological systems that can be constructed based purely on open-source data (National Hydrography Dataset and Watershed Boundary Dataset). The graph representation provides a flexible intuitive approach for capturing connectivity and for identifying upstream pollutant sources and for tracing downstream impacts within small and large hydrological systems. Moreover, the graph representation can facilitate the use of advanced algorithms and tools of graph theory, topology, optimization, and machine learning to aid data analytics and decision-making. We demonstrate the capabilities of our framework by using case studies in the State of Wisconsin; here, we aim to identify upstream nutrient pollutant sources that arise from agricultural practices and trace downstream impacts to waterbodies, rivers, and streams. Our tool ultimately seeks to help stakeholders design effective pollution prevention/mitigation practices and evaluate how surface waters respond to such practices.

References

Bauman A, Burt J, Feary D, Marquis E, Usseglio P . Tropical harmful algal blooms: an emerging threat to coral reef communities?. Mar Pollut Bull. 2010; 60(11):2117-22. DOI: 10.1016/j.marpolbul.2010.08.015. View

Soranno P, Spence Cheruvelil K, Wagner T, Webster K, Bremigan M . Effects of Land Use on Lake Nutrients: The Importance of Scale, Hydrologic Connectivity, and Region. PLoS One. 2015; 10(8):e0135454. PMC: 4534397. DOI: 10.1371/journal.pone.0135454. View

Xue J, Wang Q, Zhang M . A review of non-point source water pollution modeling for the urban-rural transitional areas of China: Research status and prospect. Sci Total Environ. 2022; 826:154146. DOI: 10.1016/j.scitotenv.2022.154146. View

Burkholder J, Libra B, Weyer P, Heathcote S, Kolpin D, Thorne P . Impacts of waste from concentrated animal feeding operations on water quality. Environ Health Perspect. 2007; 115(2):308-12. PMC: 1817674. DOI: 10.1289/ehp.8839. View

Walton C, Zak D, Audet J, Petersen R, Lange J, Oehmke C . Wetland buffer zones for nitrogen and phosphorus retention: Impacts of soil type, hydrology and vegetation. Sci Total Environ. 2020; 727:138709. DOI: 10.1016/j.scitotenv.2020.138709. View

Tasdighi A, Arabi M, Osmond D . The Relationship between Land Use and Vulnerability to Nitrogen and Phosphorus Pollution in an Urban Watershed. J Environ Qual. 2017; 46(1):113-122. DOI: 10.2134/jeq2016.06.0239. View

Ciazela J, Siepak M, Wojtowicz P . Tracking heavy metal contamination in a complex river-oxbow lake system: Middle Odra Valley, Germany/Poland. Sci Total Environ. 2017; 616-617:996-1006. DOI: 10.1016/j.scitotenv.2017.10.219. View

Oliver S, Corburn J, Ribeiro H . Challenges Regarding Water Quality of Eutrophic Reservoirs in Urban Landscapes: A Mapping Literature Review. Int J Environ Res Public Health. 2018; 16(1). PMC: 6339212. DOI: 10.3390/ijerph16010040. View

Le C, Zha Y, Li Y, Sun D, Lu H, Yin B . Eutrophication of lake waters in China: cost, causes, and control. Environ Manage. 2010; 45(4):662-8. DOI: 10.1007/s00267-010-9440-3. View

10.

Wellen C, Kamran-Disfani A, Arhonditsis G . Evaluation of the current state of distributed watershed nutrient water quality modeling. Environ Sci Technol. 2015; 49(6):3278-90. DOI: 10.1021/es5049557. View

11.

Lindim C, Van Gils J, Cousins I . A large-scale model for simulating the fate & transport of organic contaminants in river basins. Chemosphere. 2015; 144:803-10. DOI: 10.1016/j.chemosphere.2015.09.051. View

12.

Schmidt C, Kumar R, Yang S, Buttner O . Microplastic particle emission from wastewater treatment plant effluents into river networks in Germany: Loads, spatial patterns of concentrations and potential toxicity. Sci Total Environ. 2020; 737:139544. DOI: 10.1016/j.scitotenv.2020.139544. View

13.

Nawab J, Khan S, Ali S, Sher H, Rahman Z, Khan K . Health risk assessment of heavy metals and bacterial contamination in drinking water sources: a case study of Malakand Agency, Pakistan. Environ Monit Assess. 2016; 188(5):286. DOI: 10.1007/s10661-016-5296-1. View

14.

Tong X, Mohapatra S, Zhang J, Tran N, You L, He Y . Source, fate, transport and modelling of selected emerging contaminants in the aquatic environment: Current status and future perspectives. Water Res. 2022; 217:118418. DOI: 10.1016/j.watres.2022.118418. View

15.

Verhoeven J, Arheimer B, Yin C, Hefting M . Regional and global concerns over wetlands and water quality. Trends Ecol Evol. 2006; 21(2):96-103. DOI: 10.1016/j.tree.2005.11.015. View

16.

Costa C, Leite I, Almeida A, de Almeida I . Choosing an appropriate water quality model-a review. Environ Monit Assess. 2021; 193(1):38. DOI: 10.1007/s10661-020-08786-1. View

17.

Wang X, Zhang L, Zhao Z, Cai Y . Heavy metal pollution in reservoirs in the hilly area of southern China: Distribution, source apportionment and health risk assessment. Sci Total Environ. 2018; 634:158-169. DOI: 10.1016/j.scitotenv.2018.03.340. View

18.

Sampat A, Hicks A, Ruiz-Mercado G, Zavala V . Valuing economic impact reductions of nutrient pollution from livestock waste. Resour Conserv Recycl. 2021; 164. PMC: 7970505. DOI: 10.1016/j.resconrec.2020.105199. View

19.

Hobbie S, Finlay J, Janke B, Nidzgorski D, Millet D, Baker L . Contrasting nitrogen and phosphorus budgets in urban watersheds and implications for managing urban water pollution. Proc Natl Acad Sci U S A. 2017; 114(16):4177-4182. PMC: 5402417. DOI: 10.1073/pnas.1618536114. View

20.

Palla G, Derenyi I, Farkas I, Vicsek T . Uncovering the overlapping community structure of complex networks in nature and society. Nature. 2005; 435(7043):814-8. DOI: 10.1038/nature03607. View