» Articles » PMID: 38162194

Angle-resolved Photoelectron Spectroscopy in a Low-energy Electron Microscope

Overview
Journal Struct Dyn
Date 2024 Jan 1
PMID 38162194
Authors
Affiliations
Soon will be listed here.
Abstract

Spectroscopic photoemission microscopy is a well-established method to investigate the electronic structure of surfaces. In modern photoemission microscopes, the electron optics allow imaging of the image plane, momentum plane, or dispersive plane, depending on the lens setting. Furthermore, apertures allow filtering of energy-, real-, and momentum space. Here, we describe how a standard spectroscopic and low-energy electron microscope can be equipped with an additional slit at the entrance of the already present hemispherical analyzer to enable an angle- and energy-resolved photoemission mode with micrometer spatial selectivity. We apply a photogrammetric calibration to correct for image distortions of the projective system behind the analyzer and present spectra recorded on Au(111) as a benchmark. Our approach makes data acquisition in energy-momentum space more efficient, which is a necessity for laser-based pump-probe photoemission microscopy with femtosecond time resolution.

Citing Articles

Implementation and performance of a fiber-coupled CMOS camera in an ultrafast reflective high-energy electron diffraction experiment.

Fortmann J, Kassen A, Brand C, Duden T, Horn-von Hoegen M Struct Dyn. 2025; 12(2):024301.

PMID: 40060919 PMC: 11888785. DOI: 10.1063/4.0000284.

References
1.
Jobst J, Torren A, Krasovskii E, Balgley J, Dean C, Tromp R . Quantifying electronic band interactions in van der Waals materials using angle-resolved reflected-electron spectroscopy. Nat Commun. 2016; 7:13621. PMC: 5141287. DOI: 10.1038/ncomms13621. View

2.
Kevan , Gaylord . High-resolution photoemission study of the electronic structure of the noble-metal (111) surfaces. Phys Rev B Condens Matter. 1987; 36(11):5809-5818. DOI: 10.1103/physrevb.36.5809. View

3.
Sutter P, Ibragimova R, Komsa H, Parkinson B, Sutter E . Self-organized twist-heterostructures via aligned van der Waals epitaxy and solid-state transformations. Nat Commun. 2019; 10(1):5528. PMC: 6893034. DOI: 10.1038/s41467-019-13488-5. View

4.
Kromker B, Escher M, Funnemann D, Hartung D, Engelhard H, Kirschner J . Development of a momentum microscope for time resolved band structure imaging. Rev Sci Instrum. 2008; 79(5):053702. DOI: 10.1063/1.2918133. View

5.
Schmitt F, Kirchmann P, Bovensiepen U, Moore R, Rettig L, Krenz M . Transient electronic structure and melting of a charge density wave in TbTe3. Science. 2008; 321(5896):1649-52. DOI: 10.1126/science.1160778. View