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Optimization and Performance Analysis of a TiO/i-CHNHSnBr/CsPbI/Al(BSF) Heterojunction Perovskite Solar Cell for Enhanced Efficiency

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Journal ACS Omega
Specialty Chemistry
Date 2023 Oct 16
PMID 37841169
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Abstract

This paper reports the simulation and optimization of heterojunction perovskite solar cells (PSCs) with a proposed structure of TiO/i-CHNHSnBr/CsPbI/Al(BSF) using SCAPS-1D software. The purpose of this study is to investigate the performance of the PSC with CsPbI perovskite active layers and i-CHNHSnBr as the permeable layer. Therefore, the thicknesses of the layers of the heterojunction perovskite are modified in order to find a better conversion efficiency of the solar cell, where the latter's performance is improved by optimizing the absorber's thickness, which is found to be 1 μm, with a permeable layer of 15 μm. The device efficiency of the i-CHNHSnBr/CsPbI heterojunction is improved to 38.98%, and optimized parameters are = 1.21 mV, = 35.63 mA/cm, and FF = 89.84%. The acceptor concentration (), donor concentration (), defect density, and series and shunt resistances are also investigated.

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