» Articles » PMID: 36770988

Four Routes to 3-(3-Methoxy-1,3-dioxopropyl)pyrrole, a Core Motif of Rings C and E in Photosynthetic Tetrapyrroles

Overview
Journal Molecules
Publisher MDPI
Specialty Biology
Date 2023 Feb 11
PMID 36770988
Authors
Affiliations
Soon will be listed here.
Abstract

The photosynthetic tetrapyrroles share a common structural feature comprised of a β-ketoester motif embedded in an exocyclic ring (ring E). As part of a total synthesis program aimed at preparing native structures and analogues, 3-(3-methoxy-1,3-dioxopropyl)pyrrole was sought. The pyrrole is a precursor to analogues of ring C and the external framework of ring E. Four routes were developed. Routes 1-3 entail a Pd-mediated coupling process of a 3-iodopyrrole with potassium methyl malonate, whereas route 4 relies on electrophilic substitution of TIPS-pyrrole with methyl malonyl chloride. Together, the four routes afford considerable latitude. A long-term objective is to gain the capacity to create chlorophylls and bacteriochlorophylls and analogues thereof by facile de novo means for diverse studies across the photosynthetic sciences.

References
1.
Liu J, Chan H, Xue F, Wang Q, Mak T, Wong H . Generation and Trapping Reactions of 1-tert-Butoxycarbonyl-3,4-didehydro-1H-pyrrole. J Org Chem. 2001; 64(5):1630-1634. DOI: 10.1021/jo982129l. View

2.
Wang P, Chau Nguyen K, Lindsey J . Synthesis of the Ring C Pyrrole of Native Chlorophylls and Bacteriochlorophylls. J Org Chem. 2019; 84(17):11286-11293. DOI: 10.1021/acs.joc.9b01650. View

3.
Mayr H, Lakhdar S, Maji B, Ofial A . A quantitative approach to nucleophilic organocatalysis. Beilstein J Org Chem. 2012; 8:1458-78. PMC: 3458771. DOI: 10.3762/bjoc.8.166. View

4.
Meyer M, Scheer H, Breton J . Probing native-like orientation of pigments in modified reaction centers from Rhodobacter sphaeroides R26 by linear dichroism. FEBS Lett. 1996; 393(1):131-4. DOI: 10.1016/0014-5793(96)00869-1. View

5.
Frontier A, Hernandez J . New Twists in Nazarov Cyclization Chemistry. Acc Chem Res. 2020; 53(9):1822-1832. DOI: 10.1021/acs.accounts.0c00284. View