High Power Factor of AgSe/Ag/Nylon Composite Films for Wearable Thermoelectric Devices
Overview
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A flexible thermoelectric device has been considered as a competitive candidate for powering wearable electronics. Here, we fabricated an n-type AgSe/Ag composite film on a flexible nylon substrate using vacuum-assisted filtration and a combination of cold and hot pressing. By optimising the Ag/Se ratio and the sequential addition and reaction time of AA, an excellent power factor of 2277.3 μW∙m K (corresponding to a of ~0.71) at room temperature was achieved. In addition, the AgSe/Ag composite film exhibits remarkable flexibility, with only 4% loss and 10% loss in electrical conductivity after being bent around a rod of 4 mm radius for 1000 cycles and 2000 cycles, respectively. A seven-leg flexible thermoelectric device assembled with the optimised film demonstrates a voltage of 19 mV and a maximum power output of 3.48 μW (corresponding power density of 35.5 W m) at a temperature difference of 30 K. This study provides a potential path to design improved flexible TE devices.