Multiple Halide Anion Doped Layered Bismuth Terephthalate with Excellent Photocatalysis for Pollutant Removal

Overview

Journal RSC Adv

Publisher Royal Society of Chemistry

Specialty Chemistry

Date 2022 May 13

PMID 35559113

Authors

Xinyun Zhao

Huihui Chen

Xi Chen

Juncheng Hu

Tsunghsueh Wu

Lamei Wu

Mei Li

Affiliations

Soon will be listed here.

Abstract

In order to improve the photocatalytic activities of layered MOF bismuth terephthalate, five multiple halide anion doped bismuth terephthalate composites were prepared by doping three or four halide anions each with a molar ratio of X/Bi (X = F, Cl, Br, I) at 0.25. The F, Cl, Br codoped and F, Cl, Br, I codoped bismuth terephthalate composites exhibit 41 and 35 times higher photocatalytic degradation activities for RhB, 7 and 6 times higher for salicylic acid than that of bismuth terephthalate. Excellent photocatalytic activities could be ascribed to the microstructure of multiple halide anion doped composites, large specific BET surface area and effective separation of photogenerated electron-hole pairs. Incorporating multiple negatively charged F, Cl, Br, I into layered bismuth terephthalate can improve the photocatalytic and electrochemical activities of bismuth terephthalate. The composites presented in this study can be potentially applied in photocatalysis and electrochemical fields as multifunctional materials.

Citing Articles

Bismuth Coordination Polymers with Fluorinated Linkers: Aqueous Stability, Bivolatility, and Adsorptive Behavior.

Lulich A, Amiri M, Stephen D, Shohel M, Mao Z, Nyman M ACS Omega. 2023; 8(11):10476-10486.

PMID: 36969471 PMC: 10034978. DOI: 10.1021/acsomega.3c00114.

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