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Spin Transition in a Ferrous Chloride Complex Supported by a Pentapyridine Ligand

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Specialty Chemistry
Date 2020 Feb 15
PMID 32057045
Citations 1
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Abstract

Ferrous chloride complexes [FeLCl] commonly attain a high-spin state independently of the supporting ligand(s) and temperature. Herein, we present the first report of a complete spin crossover with T = 80 K in [Fe(Py5OH)Cl] (Py5OH = pyridine-2,6-diylbis[di(pyridin-2-yl)methanol]). Both spin forms of the complex are analyzed by X-ray spectroscopy and DFT calculations.

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Water Oxidation by Pentapyridyl Base Metal Complexes? A Case Study.

Boniolo M, Hossain M, Chernev P, Suremann N, Heizmann P, Lyvik A Inorg Chem. 2022; 61(24):9104-9118.

PMID: 35658429 PMC: 9214691. DOI: 10.1021/acs.inorgchem.2c00631.