Strong Hot Carrier Effects in Single Nanowire Heterostructures
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We use transient Rayleigh scattering to study the thermalization of hot photoexcited carriers in single GaAsSb/InP nanowire heterostructures. By comparing the energy loss rate in single core-only GaAsSb nanowires which do not show substantial hot carrier effects with the core-shell nanowires, we show that the presence of an InP shell substantially suppresses the longitudinal optical phonon emission rate at low temperatures which then leads to strong hot carrier effects.
Esmaielpour H, Isaev N, Makhfudz I, Doblinger M, Finley J, Koblmuller G ACS Appl Nano Mater. 2024; 7(3):2817-2824.
PMID: 38357220 PMC: 10863615. DOI: 10.1021/acsanm.3c05041.
Unraveling the Ultrafast Hot Electron Dynamics in Semiconductor Nanowires.
Wittenbecher L, Vinas Bostrom E, Vogelsang J, Lehman S, Dick K, Verdozzi C ACS Nano. 2021; 15(1):1133-1144.
PMID: 33439621 PMC: 7877729. DOI: 10.1021/acsnano.0c08101.