Room-temperature Near-infrared High-Q Perovskite Whispering-gallery Planar Nanolasers
Overview
Affiliations
Near-infrared (NIR) solid-state micro/nanolasers are important building blocks for true integration of optoelectronic circuitry. Although significant progress has been made in III-V nanowire lasers with achieving NIR lasing at room temperature, challenges remain including low quantum efficiencies and high Auger losses. Importantly, the obstacles toward integrating one-dimensional nanowires on the planar ubiquitous Si platform need to be effectively tackled. Here we demonstrate a new family of planar room-temperature NIR nanolasers based on organic-inorganic perovskite CH3NH3PbI(3-a)X(a) (X = I, Br, Cl) nanoplatelets. Their large exciton binding energies, long diffusion lengths, and naturally formed high-quality planar whispering-gallery mode cavities ensure adequate gain and efficient optical feedback for low-threshold optically pumped in-plane lasing. We show that these remarkable wavelength tunable whispering-gallery nanolasers can be easily integrated onto conductive platforms (Si, Au, indium tin oxide, and so forth). Our findings open up a new class of wavelength tunable planar nanomaterials potentially suitable for on-chip integration.
Chen Z, Shi Z, Zhang W, Li Z, Zhou Z Nanophotonics. 2024; 11(7):1379-1387.
PMID: 39634615 PMC: 11501272. DOI: 10.1515/nanoph-2021-0789.
Two-dimensional metal halide perovskites and their heterostructures: from synthesis to applications.
Kostopoulou A, Konidakis I, Stratakis E Nanophotonics. 2024; 12(9):1643-1710.
PMID: 39634119 PMC: 11501535. DOI: 10.1515/nanoph-2022-0797.
Interferometric Near-field Fano Spectroscopy of Single Halide Perovskite Nanoparticles.
Zhan J, Jehle T, Stephan S, Tiguntseva E, Nochowitz S, Gross P Nano Lett. 2024; 24(49):15738-15744.
PMID: 39609946 PMC: 11638946. DOI: 10.1021/acs.nanolett.4c04491.
Color-Tunable Lead Halide Perovskite Single-Mode Chiral Microlasers with Exceptionally High .
Gu H, Xu H, Yang C, Feng Y, Gao G, Hoye R Nano Lett. 2024; 24(42):13333-13340.
PMID: 39361829 PMC: 11503764. DOI: 10.1021/acs.nanolett.4c03838.
Lim A, Yeom T ACS Omega. 2024; 9(32):34918-34926.
PMID: 39157095 PMC: 11325393. DOI: 10.1021/acsomega.4c04606.