High-mobility Graphene on Liquid P-block Elements by Ultra-low-loss CVD Growth
Authors
Affiliations
The high-quality and low-cost of the graphene preparation method decide whether graphene is put into the applications finally. Enormous efforts have been devoted to understand and optimize the CVD process of graphene over various d-block transition metals (e.g. Cu, Ni and Pt). Here we report the growth of uniform high-quality single-layer, single-crystalline graphene flakes and their continuous films over p-block elements (e.g. Ga) liquid films using ambient-pressure chemical vapor deposition. The graphene shows high crystalline quality with electron mobility reaching levels as high as 7400 cm(2) V(-1) s(-1) under ambient conditions. Our employed growth strategy is ultra-low-loss. Only trace amounts of Ga are consumed in the production and transfer of the graphene and expensive film deposition or vacuum systems are not needed. We believe that our research will open up new territory in the field of graphene growth and thus promote its practical application.
In Situ Investigation of the Motion Behavior of Graphene on Liquid Copper.
Wang L, Ding Y, Wang X, Lai R, Zeng M, Fu L Adv Sci (Weinh). 2021; 8(17):e2100334.
PMID: 34240577 PMC: 8425870. DOI: 10.1002/advs.202100334.
Atmospheric Pressure Catalytic Vapor Deposition of Graphene on Liquid Sn and Cu-Sn Alloy Substrates.
Saeed M, Kinloch I, Derby B Nanomaterials (Basel). 2020; 10(11).
PMID: 33126626 PMC: 7692589. DOI: 10.3390/nano10112150.
Chemical Vapour Deposition of Graphene-Synthesis, Characterisation, and Applications: A Review.
Saeed M, Alshammari Y, Majeed S, Al-Nasrallah E Molecules. 2020; 25(17).
PMID: 32854226 PMC: 7503287. DOI: 10.3390/molecules25173856.
Quasi-Monocrystalline Graphene Crystallization on Liquid Copper Matrix.
Kuten D, Dybowski K, Atraszkiewicz R, Kula P Materials (Basel). 2020; 13(11).
PMID: 32521635 PMC: 7321550. DOI: 10.3390/ma13112606.
Precise Vapor-Phase Synthesis of Two-Dimensional Atomic Single Crystals.
Zhao S, Wang L, Fu L iScience. 2019; 20:527-545.
PMID: 31655063 PMC: 6818371. DOI: 10.1016/j.isci.2019.09.038.