Self-assembled Plasmonic Core-shell Clusters with an Isotropic Magnetic Dipole Response in the Visible Range

We theoretically analyze, fabricate, and characterize a three-dimensional plasmonic nanostructure that exhibits a strong and isotropic magnetic response in the visible spectral domain. Using two different bottom-up approaches that rely on self-organization and colloidal nanochemistry, we fabricate clusters consisting of dielectric core spheres, which are smaller than the wavelength of the incident radiation and are decorated by a large number of metallic nanospheres. Hence, despite having a complicated inner geometry, such a core-shell particle is sufficiently small to be perceived as an individual object in the far field. The optical properties of such complex plasmonic core-shell particles are discussed for two different core diameters.