Magnetism in Fe-based Superconductors
Overview
Biotechnology
Authors
Affiliations
In this review, we present a summary of experimental studies of magnetism in Fe-based superconductors. The doping dependent phase diagram shows strong similarities to the generic phase diagram of the cuprates. Parent compounds exhibit magnetic order together with a structural phase transition, both of which are progressively suppressed with doping, allowing superconductivity to emerge. The stripe-like spin arrangement of Fe moments in the magnetically ordered state shows identical in-plane structure for the RFeAsO (R = rare earth) and AFe(2)As(2) (A = Sr, Ca, Ba, Eu and K) parent compounds, notably different than the spin configuration of the cuprates. Interestingly, Fe(1 + y)Te orders with a different spin order despite having very similar Fermi surface topology. Studies of the spin dynamics of the parent compounds show that the interactions are best characterized as anisotropic three-dimensional interactions. Despite the room temperature tetragonal structure, analysis of the low temperature spin waves under the assumption of a Heisenberg Hamiltonian indicates strong in-plane anisotropy with a significant next-nearest-neighbor interaction. For the superconducting state, a resonance, localized in both wavevector and energy, is observed in the spin excitation spectrum as for the cuprates. This resonance is observed at a wavevector compatible with a Fermi surface nesting instability independent of the magnetic ordering of the relevant parent compound. The resonance energy (E(r)) scales with the superconducting transition temperature (T(C)) as E(r) ∼ 4.9k(B)T(C), which is consistent with the canonical value of ∼ 5k(B)T(C) observed for the cuprates. Moreover, the relationship between the resonance energy and the superconducting gap, Δ, is similar to that observed for many unconventional superconductors (E(r)/2Δ ∼ 0.64).
Kim M, Ratcliff 2nd W, Pajerowski D, Kim J, Yan J, Lynn J Phys Rev B. 2023; 103(17).
PMID: 37588030 PMC: 10428661. DOI: 10.1103/physrevb.103.174405.
Direct Observation of the Spin Exciton in Andreev Spectroscopy of Iron-Based Superconductors.
Korshunov M, Kuzmichev S, Kuzmicheva T Materials (Basel). 2022; 15(17).
PMID: 36079499 PMC: 9458014. DOI: 10.3390/ma15176120.
Band Structure of Organic-Ion-Intercalated (EMIM)FeSe Superconductor.
Begunovich L, Korshunov M Materials (Basel). 2022; 15(5).
PMID: 35269087 PMC: 8911679. DOI: 10.3390/ma15051856.
Iron pnictides and chalcogenides: a new paradigm for superconductivity.
Fernandes R, Coldea A, Ding H, Fisher I, Hirschfeld P, Kotliar G Nature. 2022; 601(7891):35-44.
PMID: 34987212 DOI: 10.1038/s41586-021-04073-2.
Spin dynamics of the block orbital-selective Mott phase.
Herbrych J, Kaushal N, Nocera A, Alvarez G, Moreo A, Dagotto E Nat Commun. 2018; 9(1):3736.
PMID: 30213941 PMC: 6137186. DOI: 10.1038/s41467-018-06181-6.