Supercycled Homonuclear Dipolar Decoupling Sequences in Solid-state NMR

We compare the performance of the windowed phase-modulated Lee-Goldburg (wPMLG) and the windowed decoupling using mind boggling optimisation (wDUMBO) sequences at various magic-angle spinning rates and nutation frequencies of the pulses. Additionally, we introduce a supercycled version of wDUMBO and compare its efficiency with that of the non-supercycled implementation of wDUMBO. The efficiency of the supercycled version of wPMLG, denoted wPMLG-S2, is compared with a new supercycled version of wPMLG that we notate as wPMLG-S3. The interaction between the supercycled homonuclear dipolar decoupling sequences and the sample rotation is analysed using symmetry-based selection rules.